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Official PDF TranslationChinese Traditional and Herbal Drugs

UPLC-MS/MS Metabolomics Profiling of Differential Chemical Constituents and Blood-Absorbed Components Between Raw and Steamed Rhei Radix et Rhizoma

Authors: XIA Xuejie; SUN Shuding; LIU Xuefang; ZHAO Di; LI Rongrong; FENG Suxiang

DOI: 10.7501/j.issn.0253-2670.2026.16.20261604Status: Verified Translated Edition
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Key Findings in This Report

• • Steaming significantly upregulated 7 constituents (P < 0.05), including chrysophanol, gallic acid, and catechin, while downregulating 16 constituents (P < 0.05), including aloe-emodin-1-O-β-D-glucopyranoside, sennoside A, and proanthocyanidins, among 201 identified compounds; this shift underpins the reduced purgative potency and enhanced blood-activating efficacy of steamed Rhei Radix et Rhizoma in clinical practice. • • Serum pharmacochemistry identified 94 migrated components (36 prototypes, 58 metabolites) with 11 differential constituents between raw and steamed preparations; steamed Rhei Radix et Rhizoma showed elevated serum levels of gallic acid and phase-II anthraquinone metabolites, indicating enhanced glucuronidation and accelerated excretion of emodin and rhein, which mechanistically explains the attenuated hepatotoxicity observed after processing. • • The conversion of bound anthraquinones to free aglycones in steamed Rhei Radix et Rhizoma increases the bioavailability of emodin and rhein, yielding a synergistic potentiation effect; this transformation supports the clinical preference for steamed Rhei Radix et Rhizoma in elderly, pediatric, and postpartum patients requiring purgation without severe depletion of vital qi. • • Depolymerization of hydrolyzable tannins into monomeric gallic acid and dynamic interconversion between condensed tannins and flavonoid aglycones were observed, providing a chemical basis for the enhanced blood-activating and stasis-dissipating properties of steamed Rhei Radix et Rhizoma; these markers can serve as quality control indicators for processing standardization.